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Get Free AccessWe compare the results from time-resolved fluorescence anisotropy experiments and molecular modelling on perylene bisimide acrylate dimers which allows us to connect the observed spectral signatures unambiguously with the non-stacked and two (parallel and anti-parallel) stacked conformations. For the parallel stacked conformation the experimental data can be reproduced quantitatively using a model that assumes structural relaxation in the electronically excited state of the stacked aggregate. For the non-stacked conformation we find quantitative agreement between experiment and modelling only if a fast hopping of the electronic excitation between the perylene bisimide subunits is taken into account.
Florian Spreitler, Michael Sommer, M. Hollfelder, Mukundan Mukundan Thelakkat, Stephan Gekle, Jürgen Köhler (2014). Unravelling the conformations of di-(perylene bisimide acrylate) by combining time-resolved fluorescence-anisotropy experiments and molecular modelling. , 16(47), DOI: https://doi.org/10.1039/c4cp03064h.
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Type
Article
Year
2014
Authors
6
Datasets
0
Total Files
0
Language
en
DOI
https://doi.org/10.1039/c4cp03064h
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