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  5. Quasiparticle Gap Renormalization Driven by Internal and External Screening in a <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>WS</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math> Device

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Article
lv
2025

Quasiparticle Gap Renormalization Driven by Internal and External Screening in a <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>WS</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math> Device

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lv
2025
Vol 135 (5)
Vol. 135
DOI: 10.1103/yllv-5zx7

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Kenji Watanabe
Kenji Watanabe

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Yann in ’t Veld
Alfred J. H. Jones
Zhihao Jiang
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Abstract

The electronic band gap of a two-dimensional semiconductor within a device architecture is sensitive to variations in screening properties of adjacent materials in the device and to gate-controlled doping. Here, we employ microfocused angle-resolved photoemission spectroscopy to separate band gap renormalization effects stemming from environmental screening and electron doping during in situ gating of a single-layer WS_{2} device. The WS_{2} is supported on hexagonal boron nitride and contains a section that is exposed to vacuum and another section that is encapsulated by a graphene contact. We directly observe the doping-induced semiconductor-metal transition and band gap renormalization in the two sections of WS_{2}. Surprisingly, a larger band gap renormalization is observed in the vacuum-exposed section than in the graphene-encapsulated-and thus ostensibly better screened-section of the WS_{2}. Using GW calculations, we determine that intrinsic screening due to stronger doping in vacuum-exposed WS_{2} exceeds the external environmental screening in graphene-encapsulated WS_{2}.

How to cite this publication

Yann in ’t Veld, Alfred J. H. Jones, Zhihao Jiang, Greta Lupi, Paulina Majchrzak, Kimberly Hsieh, Kenji Watanabe, Takashi Taniguchi, Philip Hofmann, Jill A. Miwa, Yong P. Chen, Malte Rösner, Søren Ulstrup (2025). Quasiparticle Gap Renormalization Driven by Internal and External Screening in a <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>WS</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math> Device. , 135(5), DOI: https://doi.org/10.1103/yllv-5zx7.

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Publication Details

Type

Article

Year

2025

Authors

13

Datasets

0

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0

Language

lv

DOI

https://doi.org/10.1103/yllv-5zx7

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