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  5. Origin of Nonlinear Circular Photocurrent in 2D Semiconductor <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>MoS</mml:mi></mml:mrow><mml:mn>2</mml:mn></mml:msub></mml:mrow></mml:math>

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Article
lv
2025

Origin of Nonlinear Circular Photocurrent in 2D Semiconductor <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>MoS</mml:mi></mml:mrow><mml:mn>2</mml:mn></mml:msub></mml:mrow></mml:math>

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lv
2025
Vol 134 (8)
Vol. 134
DOI: 10.1103/physrevlett.134.086201

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Kenji Watanabe
Kenji Watanabe

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Yanchong Zhao
Fengyu Chen
Jing Liang
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Abstract

Nonlinear photogalvanic effects in two-dimensional materials, particularly the nonlinear circular photocurrents (NCPs) that belong to the helicity-dependent spin photocurrents, have sparked enormous research interest. Although notable progress has been witnessed, the underling origin of NCPs remains elusive. Here, we present systematic photocurrent characteristics, symmetry analysis and theoretical calculations to uncover the physical origin of NCPs in MoS_{2}, a prototypical 2D semiconductor. Our results show that the NCP responses in 2D semiconductor MoS_{2} result from the circular photon drag effect (CPDE), rather than the generally believed circular photogalvanic effect. Furthermore, we demonstrate that the NCPs are highly tunable with electrostatic doping and increase progressively with MoS_{2} thickness, evidencing the interlayer constructive nature of CPDE responses. Our Letter unravels the critical role of the previously overlooked CPDE contribution to NCPs, revolutionizing previous understanding and thus providing deep insights into further fundamental studies and technological advances in nonlinear photovoltaic and opto-spintronic devices.

How to cite this publication

Yanchong Zhao, Fengyu Chen, Jing Liang, M. S. Bahramy, Ming‐Wei Yang, Guang Yao, Xiaomei Li, Wei Zheng, Jianhui Tang, Jiaojiao Zhao, Mengzhou Liao, Cheng Shen, Qinqin Wang, Rong Yang, Kenji Watanabe, Takashi Taniguchi, Zhiheng Huang, Dongxia Shi, Kaihui Liu, Zhipei Sun, Ji Feng, Luojun Du, Guangyu Zhang (2025). Origin of Nonlinear Circular Photocurrent in 2D Semiconductor <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>MoS</mml:mi></mml:mrow><mml:mn>2</mml:mn></mml:msub></mml:mrow></mml:math>. , 134(8), DOI: https://doi.org/10.1103/physrevlett.134.086201.

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Publication Details

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Article

Year

2025

Authors

23

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0

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Language

lv

DOI

https://doi.org/10.1103/physrevlett.134.086201

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