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Get Free AccessNonlinear photogalvanic effects in two-dimensional materials, particularly the nonlinear circular photocurrents (NCPs) that belong to the helicity-dependent spin photocurrents, have sparked enormous research interest. Although notable progress has been witnessed, the underling origin of NCPs remains elusive. Here, we present systematic photocurrent characteristics, symmetry analysis and theoretical calculations to uncover the physical origin of NCPs in MoS_{2}, a prototypical 2D semiconductor. Our results show that the NCP responses in 2D semiconductor MoS_{2} result from the circular photon drag effect (CPDE), rather than the generally believed circular photogalvanic effect. Furthermore, we demonstrate that the NCPs are highly tunable with electrostatic doping and increase progressively with MoS_{2} thickness, evidencing the interlayer constructive nature of CPDE responses. Our Letter unravels the critical role of the previously overlooked CPDE contribution to NCPs, revolutionizing previous understanding and thus providing deep insights into further fundamental studies and technological advances in nonlinear photovoltaic and opto-spintronic devices.
Yanchong Zhao, Fengyu Chen, Jing Liang, M. S. Bahramy, Ming‐Wei Yang, Guang Yao, Xiaomei Li, Wei Zheng, Jianhui Tang, Jiaojiao Zhao, Mengzhou Liao, Cheng Shen, Qinqin Wang, Rong Yang, Kenji Watanabe, Takashi Taniguchi, Zhiheng Huang, Dongxia Shi, Kaihui Liu, Zhipei Sun, Ji Feng, Luojun Du, Guangyu Zhang (2025). Origin of Nonlinear Circular Photocurrent in 2D Semiconductor <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>MoS</mml:mi></mml:mrow><mml:mn>2</mml:mn></mml:msub></mml:mrow></mml:math>. , 134(8), DOI: https://doi.org/10.1103/physrevlett.134.086201.
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Type
Article
Year
2025
Authors
23
Datasets
0
Total Files
0
Language
lv
DOI
https://doi.org/10.1103/physrevlett.134.086201
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