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Get Free AccessNear-monodisperse Ni{sub 1-x}Cu{sub x} (x = 0.2-0.8) bimetallic nanocrystals were synthesized by a one-pot thermolysis approach in oleylamine/1-octadecene, using metal acetylacetonates as precursors. The nanocrystals form large-area 2D superlattices, and display a catalytic synergistic effect in the hydrolysis of NaBH{sub 4} to generate H{sub 2} at x = 0.5 in a strongly basic medium. The Ni{sub 0.5}Cu{sub 0.5} nanocrystals show the lowest activation energy, and also exhibit the highest H{sub 2} generation rate at 298 K.
Ya‐Wen Zhang, Wenyu Huang, Susan E. Habas, John N. Kuhn, Michael Graß, Yusuke Yamada, Peidong Yang, Gabor Somorjai (2008). Near-Monodisperse Ni−Cu Bimetallic Nanocrystals of Variable Composition: Controlled Synthesis and Catalytic Activity for H<sub>2</sub> Generation. , 112(32), DOI: https://doi.org/10.1021/jp805788x.
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Type
Article
Year
2008
Authors
8
Datasets
0
Total Files
0
Language
en
DOI
https://doi.org/10.1021/jp805788x
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