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Get Free AccessMoTe_{2} monolayers and bilayers are unique within the family of van der Waals materials since they pave the way toward atomically thin infrared light-matter quantum interfaces, potentially reaching the important telecommunication windows. Here, we report emergent exciton polaritons based on MoTe_{2} monolayers and bilayers in a low-temperature open microcavity in a joint experiment-theory study. Our experiments clearly evidence both the enhanced oscillator strength and enhanced luminescence of MoTe_{2} bilayers, signified by a 38% increase of the Rabi splitting and a strongly enhanced relaxation of polaritons to low-energy states. The latter is distinct from polaritons in MoTe_{2} monolayers, which feature a bottlenecklike relaxation inhibition. Both the polaritonic spin valley locking in monolayers and the spin-layer locking in bilayers are revealed via the Zeeman effect, which we map and control via the light-matter composition of our polaritonic resonances.
Bo Han, Jamie M. Fitzgerald, Lukas Lackner, Roberto Rosati, Martin Esmann, Falk Eilenberger, Takashi Taniguchi, Kenji Watanabe, M. Syperek, Ermin Malić, Christian Schneider (2025). Infrared Magnetopolaritons in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>MoTe</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math> Monolayers and Bilayers. , 134(7), DOI: https://doi.org/10.1103/physrevlett.134.076902.
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Type
Article
Year
2025
Authors
11
Datasets
0
Total Files
0
Language
en
DOI
https://doi.org/10.1103/physrevlett.134.076902
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