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Get Free AccessHerein is reported the direct asymmetric addition of phenol nucleophiles to benzopyrylium salts as a means to produce enantioenriched flavonoid-like compounds. This enantioselective C-C bond construction was achieved through a chiral anion phase-transfer strategy that mimics the proposed biosynthesis of this structurally diverse set of natural products. The utility of this methodology was demonstrated in enantioselective synthesis of a 2,8-dioxabicyclo[3.3.1]nonane and a 2,4-diarylbenzopyran.
Zhen‐Yu Yang, Ying He, Dean Toste (2016). Biomimetic Approach to the Catalytic Enantioselective Synthesis of Flavonoids. , 138(31), DOI: https://doi.org/10.1021/jacs.6b05939.
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Type
Article
Year
2016
Authors
3
Datasets
0
Total Files
0
Language
en
DOI
https://doi.org/10.1021/jacs.6b05939
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