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Get Free AccessSignificance Using a supramolecular assembly that catalyzes substrates in water, we show that the nanocage encapsulates a water cluster that is structurally and dynamically distinct from any known phase of water. It plays an important role in the driving force for guest encapsulation: The release of the highly unusual encapsulated water droplet creates a strong thermodynamic drive for the high-affinity binding of guests in aqueous solution for the supramolecular construct.
Federico Sebastiani, Trandon A. Bender, Simone Pezzotti, Wan‐Lu Li, Gerhard Schwaab, Robert G. Bergman, Kenneth N. Raymond, Dean Toste, Teresa Head‐Gordon, Stefan Henkel (2020). An isolated water droplet in the aqueous solution of a supramolecular tetrahedral cage. , 117(52), DOI: https://doi.org/10.1073/pnas.2012545117.
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Type
Preprint
Year
2020
Authors
10
Datasets
0
Total Files
0
Language
en
DOI
https://doi.org/10.1073/pnas.2012545117
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